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  1. Radiocarbon (14C) is a critical tool for understanding the global carbon cycle. During the Anthropocene, two new processes influenced14C in atmospheric, land and ocean carbon reservoirs. First,14C-free carbon derived from fossil fuel burning has diluted14C, at rates that have accelerated with time. Second, ‘bomb’14C produced by atmospheric nuclear weapon tests in the mid-twentieth century provided a global isotope tracer that is used to constrain rates of air–sea gas exchange, carbon turnover, large-scale atmospheric and ocean transport, and other key C cycle processes. As we write, the14C/12C ratio of atmospheric CO2is dropping below pre-industrial levels, and the rate of decline in the future will depend on global fossil fuel use and net exchange of bomb14C between the atmosphere, ocean and land. This milestone coincides with a rapid increase in14C measurement capacity worldwide. Leveraging future14C measurements to understand processes and test models requires coordinated international effort—a ‘decade of radiocarbon’ with multiple goals: (i) filling observational gaps using archives, (ii) building and sustaining observation networks to increase measurement density across carbon reservoirs, (iii) developing databases, synthesis and modelling tools and (iv) establishing metrics for identifying and verifying changes in carbon sources and sinks.

    This article is part of the Theo Murphy meeting issue 'Radiocarbon in the Anthropocene'.

     
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    Free, publicly-accessible full text available November 27, 2024
  2. Abstract The Sun sporadically produces eruptive events leading to intense fluxes of solar energetic particles (SEPs) that dramatically disrupt the near-Earth radiation environment. Such events have been directly studied for the last decades but little is known about the occurrence and magnitude of rare, extreme SEP events. Presently, a few events that produced measurable signals in cosmogenic radionuclides such as 14 C, 10 Be and 36 Cl have been found. Analyzing annual 14 C concentrations in tree-rings from Switzerland, Germany, Ireland, Russia, and the USA we discovered two spikes in atmospheric 14 C occurring in 7176 and 5259 BCE. The ~2% increases of atmospheric 14 C recorded for both events exceed all previously known 14 C peaks but after correction for the geomagnetic field, they are comparable to the largest event of this type discovered so far at 775 CE. These strong events serve as accurate time markers for the synchronization with floating tree-ring and ice core records and provide critical information on the previous occurrence of extreme solar events which may threaten modern infrastructure. 
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